I'm coming from a teacher's standpoint rather than that of a student, so my perspective may be a little different, but I have very strong opinions in this area (and most of my students have agreed). Far and away, the best overall TOEFL book to me is "The Complete Guide to the TOEFL Test -- iBT Edition" by Bruce Rogers, published by Thomson. It's not the easiest to find (especially to get the self-study pack with the book, CD ROM, 13 audio Cds, and answer book), but I think it's "head and shoulders" above the rest, both in terms of quality and quantity (it's over 800 pages with 13 audio CDs!!).
I've used many others, though, and they all have strengths and weaknesses. The biggest problem I've found with most of them is that they don't represent the material correctly -- especially the integrated witing and some of the integrated speaking tasks. This could be said for the Barron's book (especially their integrated writing and several task 4's on the speaking), Delta Keys, Cambridge, Longman, Princeton Review, and Kaplan.
For example, just take Speaking Task 5, the problem/solution task. If you practiced this from the Delta, you would expect three solutions most of the time from conversation rather than 2, and if you used the Longman, you wouldn't even know that they will ask for your own opinion in addition to the summarizing of the problem and solution (unless they've finally corrected this in the most recent edition). This is just one example, but many of these books are loaded with problems.
The ETS Guide is very good, but there isn't really much study material (less than 400 pages and only 1 CD with one set of listening tasks, speaking files, etc.).
Best of luck to you in your studies, whichever book or books you use!
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